High mobility indium zinc oxide thin film field-effect transistors by semiconductor layer engineering.
Identifieur interne : 000D41 ( Main/Exploration ); précédent : 000D40; suivant : 000D42High mobility indium zinc oxide thin film field-effect transistors by semiconductor layer engineering.
Auteurs : RBID : pubmed:23163608Abstract
Indium zinc oxide thin-film transistors are fabricated via a precursor in solution route on silicon substrates with silicon dioxide gate dielectric. It is found that the extracted mobility rises, peaks, and then decreases with increasing precursor concentration instead of rising and saturating. Investigation with scanning probe techniques reveals full thickness variations within the film which are assumed to adversely affect charge transport. Additional layers are coated, and the extracted mobility is observed to increase up to 19.7 cm(2) V(-1) s(-1). The reasons for this are examined in detail by direct imaging with scanning tunneling microscopy and extracting electron density profiles from X-ray reflection measurements. It is found that the optimal concentration for single layer films is suboptimal when coating multiple layers and in fact using many layers of very low concentrations of precursor in the solution, leading to a dense, defect and void free film, affording the highest mobilities. A consistent qualitative model of layer formation is developed explaining how the morphology of the film develops as the concentration of precursor in the initial solution is varied.
DOI: 10.1021/am302004j
PubMed: 23163608
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Le document en format XML
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<author><name sortKey="Walker, Daniel E" uniqKey="Walker D">Daniel E Walker</name>
<affiliation wicri:level="3"><nlm:affiliation>Technical University of Darmstadt, Department of Materials Science, 64287 Darmstadt, Germany. walker@e-mat.tu-darmstadt.de</nlm:affiliation>
<country xml:lang="fr">Allemagne</country>
<wicri:regionArea>Technical University of Darmstadt, Department of Materials Science, 64287 Darmstadt</wicri:regionArea>
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<author><name sortKey="Major, Marton" uniqKey="Major M">Marton Major</name>
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<author><name sortKey="Yazdi, Mehrdad Baghaie" uniqKey="Yazdi M">Mehrdad Baghaie Yazdi</name>
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<author><name sortKey="Klyszcz, Andreas" uniqKey="Klyszcz A">Andreas Klyszcz</name>
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<author><name sortKey="Haeming, Marc" uniqKey="Haeming M">Marc Haeming</name>
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<author><name sortKey="Bonrad, Klaus" uniqKey="Bonrad K">Klaus Bonrad</name>
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<author><name sortKey="Melzer, Christian" uniqKey="Melzer C">Christian Melzer</name>
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<author><name sortKey="Donner, Wolfgang" uniqKey="Donner W">Wolfgang Donner</name>
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<author><name sortKey="Von Seggern, Heinz" uniqKey="Von Seggern H">Heinz von Seggern</name>
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<front><div type="abstract" xml:lang="en">Indium zinc oxide thin-film transistors are fabricated via a precursor in solution route on silicon substrates with silicon dioxide gate dielectric. It is found that the extracted mobility rises, peaks, and then decreases with increasing precursor concentration instead of rising and saturating. Investigation with scanning probe techniques reveals full thickness variations within the film which are assumed to adversely affect charge transport. Additional layers are coated, and the extracted mobility is observed to increase up to 19.7 cm(2) V(-1) s(-1). The reasons for this are examined in detail by direct imaging with scanning tunneling microscopy and extracting electron density profiles from X-ray reflection measurements. It is found that the optimal concentration for single layer films is suboptimal when coating multiple layers and in fact using many layers of very low concentrations of precursor in the solution, leading to a dense, defect and void free film, affording the highest mobilities. A consistent qualitative model of layer formation is developed explaining how the morphology of the film develops as the concentration of precursor in the initial solution is varied.</div>
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<Abstract><AbstractText>Indium zinc oxide thin-film transistors are fabricated via a precursor in solution route on silicon substrates with silicon dioxide gate dielectric. It is found that the extracted mobility rises, peaks, and then decreases with increasing precursor concentration instead of rising and saturating. Investigation with scanning probe techniques reveals full thickness variations within the film which are assumed to adversely affect charge transport. Additional layers are coated, and the extracted mobility is observed to increase up to 19.7 cm(2) V(-1) s(-1). The reasons for this are examined in detail by direct imaging with scanning tunneling microscopy and extracting electron density profiles from X-ray reflection measurements. It is found that the optimal concentration for single layer films is suboptimal when coating multiple layers and in fact using many layers of very low concentrations of precursor in the solution, leading to a dense, defect and void free film, affording the highest mobilities. A consistent qualitative model of layer formation is developed explaining how the morphology of the film develops as the concentration of precursor in the initial solution is varied.</AbstractText>
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